Magneto-electric ceramic composites are important materials for designing new microwave sensors. Keywords: Magneto-Electric Composites, Powder X-ray diffraction (PXRD), Scanning Electron Microscopy (SEM), Energy Dispersive X-ray Spectroscopy (EDS), UV-Visible Spectrophotometry (UV-Vis), Electrical (Dielectric and P-E) Characterization, Magnetic Characterization (M-H), Structural Parameters, Morphological Studies, Elementary Analysis, Optical Studies, Electrical Studies, Magnetic Studies, Charge Density Analysis.